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Mechanisms and controlling characteristics of the catalytic oxidation of methane [electronic resource].

Published:
Washington, D.C. : United States. Dept. of Energy, 1990.
Oak Ridge, Tenn. : Distributed by the Office of Scientific and Technical Information, U.S. Dept. of Energy.
Physical Description:
Pages: (15 pages) : digital, PDF file
Additional Creators:
United States. Department of Energy and United States. Department of Energy. Office of Scientific and Technical Information
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Summary:
Progress has included (1) construction and installation of an ultraviolet photoelectron spectrometer (UPS) with power supply and pumping system that has been added as an attachment to the SCIENTA ESCA-300 instrument, (2) modification of the high resolution electron energy loss spectrometer (HREELS) to produce a stable ultra high vacuum (UHV) environment for initial experiments with a Pd(311) single crystal, (3) construction of a separate high vacuum system for preparation of surface doped model catalysts by chemical vapor deposition and pretreatment of a Pd(100) single crystal in this system, (4) carried out detailed experiments of methane activation and oxidation on Pd(679) using a high pressure reaction cell contained in a third ultra high vacuum system, (5) completion of adsorption/desorption studies of H₂, CO, and O₂ on Pd(679), (6) utilized angle-resolved XPS to probe the diffraction characteristics and structure of the Pd(100) surface, (7) determination of the electronic surface structure of Pd(100) using angle-resolved UPS, and (8) computational analysis of oxygen overlayers on the PD(100) surface. Each of these is discussed in further detail below.
Report Numbers:
E 1.99:doe/er/13580-2
doe/er/13580-2
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Note:
Published through SciTech Connect.
01/01/1990.
"doe/er/13580-2"
"DE92008232"
Klier, K.
Lehigh Univ., Bethlehem, PA (United States)
Funding Information:
FG02-86ER13580
View MARC record | catkey: 14396488